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The O + NO( v) Vibrational Relaxation Processes Revisited.
Journal of Physical Chemistry. A 2018 June 22
We have carried out a quasiclassical trajectory study of the O + NO( v) energy transfer process using DMBE potential energy surfaces for the ground-states of the 2 A' and 2 A″ manifolds. State-to-state vibrational relaxation rate constants have been computed over the temperature range 298 and 3000 K and initial vibrational states between v = 1 and 9. The momentum-Gaussian binning approach has been employed to calculate the probability of the vibrational transitions. A comparison of the calculated state-to-state rate coefficients with the results from experimental studies and previous theoretical calculations shows the relevance of the 1 2 A″ potential energy surface to the title vibrational relaxation process.
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