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Evidence of symmetry breaking in a Gd 2 di-nuclear molecular polymer.
Physical Chemistry Chemical Physics : PCCP 2023 Februrary 14
A chiral 3D coordination compound, [Gd2 (L)2 (ox)2 (H2 O)2 ], arranged around a dinuclear Gd unit has been characterized by X-ray photoemission and X-ray absorption measurements in the context of density functional theory studies. Core level photoemission of the Gd 5p multiplet splittings indicates that spin orbit coupling dominates over j-J coupling evident in the 5p core level spectra of Gd metal. Indications of spin-orbit coupling are consistent with the absence of inversion symmetry due to the ligand field. Density functional theory predicts antiferromagnet alignment of the Gd2 dimers and a band gap of the compound consistent with optical absorption.
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