Measurement of 232 Th and 238 U neutron capture cross-sections in the energy range 5-17 MeV.

The neutron capture cross sections of 232 Th and 238 U at the average neutron energies of 5.08 ± 0.17, 8.96 ± 0.77, 12.47 ± 0.83, and 16.63 ± 0.95 MeV have been measured by using the activation technique and off-line γ-ray spectroscopy. The 232 Th and 238 U were irradiated with neutrons produced from the 7 Li(p, n) reaction using the proton energies of 7, 11, 15 and 18.8 MeV from the 14UD BARC-TIFR Pelletron facility in Mumbai, India. Detailed covariance analysis was also performed to evaluate the uncertainties in the measured cross-sections. The excitation function of the 232 Th(n, γ) and 238 U(n, γ) reactions were calculated using the theoretical model code TALYS-1.9. The experimental and theoretical results from the present work were compared with the ENDF/B-VII-1 and JENDL-4.0 nuclear data libraries and were found to be in good agreement.