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The gold(iii)-CO bond: a missing piece in the gold carbonyl complex landscape.
Chemical Communications : Chem Comm 2017 Februrary 5
We investigate the Au(iii)-CO bond in the [(C∧ N∧ C)Au(iii)CO]+ complex via charge-displacement (CD) analysis, revealing surprising peculiarities with respect to the Au(i)-CO bond. It shows a large Au(iii) ← CO σ donation and, unexpectedly, an even larger Au(iii) → CO π back-donation. The overall bonding picture, including a marked anisotropy in the Au(iii) → CO in-plane and out-of-plane π back-donation components, is consistent with a CO carbon atom highly susceptible to nucleophilic attack.
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