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Dynamic covalent single chain nanoparticles based on hetero Diels-Alder chemistry.

Nils Wedler-Jasinski, Thorsten Lueckerath, Hatice Mutlu, Anja S Goldmann, Andreas Walther, Martina H Stenzel, Christopher Barner-Kowollik
Chemical Communications : Chem Comm 2016 December 21
We introduce the fully reversible folding of single chain nanoparticles (SCNPs) based on covalent hetero Diels-Alder (HDA) chemistry. A cyclopentadiene (Cp)-protected cyanodithioester (CDTE) monomer is designed and copolymerized with methyl methacrylate (MMA) via RAFT polymerization. The polymer chains are folded and subsequently unfolded by exploiting the reversible nature of the HDA reaction.

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