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Multifaceted magnetization dynamics in the mononuclear complex [Re IV Cl 4 (CN) 2 ] 2 .

Xiaowen Feng, Jun-Liang Liu, Kasper S Pedersen, Joscha Nehrkorn, Alexander Schnegg, Karsten Holldack, Jesper Bendix, Marc Sigrist, Hannu Mutka, Dumitru Samohvalov, David Aguilà, Ming-Liang Tong, Jeffrey R Long, Rodolphe Clérac
Chemical Communications : Chem Comm 2016 October 26
The mononuclear complex (Bu4 N)2 [ReIV Cl4 (CN)2 ]·2DMA (DMA = N,N-dimethylacetamide) displays intricate magnetization dynamics, implying Orbach, direct, and Raman-type relaxation processes. The Orbach relaxation process is characterized by an energy barrier of 39 K (27 cm-1 ) that is discussed based on high-field electron paramagnetic resonance (EPR), inelastic neutron scattering and frequency-domain THz EPR investigations.

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