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Chemical Ligation-Mediated Total Synthesis of Corramycin.
Organic Letters 2024 April 3
The ligation-mediated total synthesis of corramycin, a myxobacterial natural product of the strain Corallococcus coralloides , is presented. The synthetic strategy included using two consecutive chemical ligations for a modular and efficient preparation. Finally, the synthesis employed a Ser/Thr ligation (STL) at a new ligation site combined with classical fragment coupling. This study provides the total synthesis of corramycin and enhances the preparative toolbox of STL in organic synthesis.
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