Electrically tunable Feshbach resonances in twisted bilayer semiconductors.

Moiré superlattices in transition metal dichalcogenide bilayers provide a platform for exploring strong correlations with optical spectroscopy. Despite the observation of rich Mott-Wigner physics stemming from an interplay between the periodic potential and Coulomb interactions, the absence of tunnel coupling–induced hybridization of electronic states has ensured a classical layer degree of freedom. We investigated a MoSe2 homobilayer structure where interlayer coherent tunneling allows for electric field–controlled manipulation and measurement of the ground-state hole-layer pseudospin. We observed an electrically tunable two-dimensional Feshbach resonance in exciton-hole scattering, which allowed us to control the strength of interactions between excitons and holes located in different layers. Our results may enable the realization of degenerate Bose-Fermi mixtures with tunable interactions.