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Novel metal-organic frameworks with high stability for selectively sensing nitroaromatics.

The stability and functionality of metal-organic frameworks (MOFs) are particularly important in considering their potential and/or practical use. Herein we report two novel aldehyde functional group-containing MOFs [Zn2 (L)(BDC)2 ]·2DMF·MeOH·H2 O (1) and [Co2 (L)(BDC)2 ]·2DMF·2MeOH·H2 O (2) (DMF = N,N-dimethylformamide, MeOH = methanol) achieved by reactions of mixed organic ligands of 2,4-bis[(pyridin-4-yl)methoxy]benzaldehyde (L) and 1,4-benzenedicarboxylic acid (H2 BDC) with the corresponding metal salts under solvothermal conditions. Both 1 and 2 are 2-fold interpenetrated three-dimensional (3D) frameworks. Particularly, 1 exhibits excellent water and wide-range pH stability, and a large Qst value for carbon dioxide (CO2 ) adsorption. Furthermore, photoluminescence (PL) studies indicate that 1 could be considered as a potential luminescent probe for detection of nitroaromatics.

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