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Intense yellow luminescence from Dy 3+ -doped TeO 2 -WO 3 -GeO 2 glasses: structural and optical characterization.
Different concentrations of Dy3+ -doped oxyfluoride tellurite (TWGDy) glasses of composition (85 - x) TeO2 + 5 WO3 + 10 GeO2 + x DyF3 , where x = 0, 0.1, 0.5, 1.0 and 2.0 mol% were prepared by melt quenching method. The Judd-Ofelt theory was applied to study the luminescence properties. Three phenomenological Judd-Ofelt (Ω λ=2,4,6 ) intensity parameters were obtained as Ω2 = 4.90 × 10-20 cm2 , Ω4 = 1.73 × 10-20 cm2 and Ω6 = 1.48 × 10-20 cm2 for 0.5 mol% of Dy3+ -doped TWGDy glass. When excited at different wavelengths, the TWGDy glasses exhibit three emission bands due to 4 F9/2 → 6 H15/2 (blue), 4 F9/2 → 6 H13/2 (yellow) and 4 F9/2 → 6 H11/2 (red) transitions. The excitation wavelength was optimized as 453 nm for strong and proficient luminescence from TWGDy glasses. Beyond 0.5 mol% of Dy3+ concentration, the TWGDy glasses show luminescence quenching. The laser characteristic parameters such as effective bandwidth, stimulated emission cross-section, gain bandwidth and optical gain were determined using the emission spectra and radiative parameters. The 0.5 mol% of Dy3+ -doped TWGDy glass could be potential to design a new class of yellow laser material.
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