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On the dual reactivity of a Janus-type mesoionic dipole: experiments and theoretical validation.
Organic & Biomolecular Chemistry 2018 July 5
A mesoionic bicycle, easily synthesized from a proteinogenic amino acid, l-leucine, behaves as both thiazolium-olate and diazolium-olate dipoles, as unveiled by its dipolar cycloadditions. This chameleonic reactivity has been thoroughly interpreted by dissecting the mechanistic landscape aided by the distortion-interaction model.
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