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Journal Article
Research Support, Non-U.S. Gov't
Total Syntheses of Pusilatins A-C, Liverwort-Derived Macrocyclic Bisbibenzyl Dimers.
Organic Letters 2018 June 16
The total syntheses of pusilatins A (2), B (3), and C (5), macrocyclic bisbibenzyl dimers isolated from Japanese liverwort are reported. The common monomeric unit (6) was prepared via macrocyclization of an o-sulfinylfluorobenzene derivative by SN Ar attack of an internal phenol, which was exploited for site-selective dimerizations en route to 2, 3, and 5.
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