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Photocatalytic difunctionalisations of alkenes with N-SCN sulfoximines.

Duo Zhang, Han Wang, Carsten Bolm
Chemical Communications : Chem Comm 2018 May 32
Reacting N-Br sulfoximines with ammonium thiocyanate leads to unprecedented sulfur reagents, which add to vinyl arenes under photocatalysis via N-centered sulfoximidoyl radicals. As a result, 1,2-difunctionalised products are obtained, which can subsequently be derivatised taking advantage of the unique properties of the thiocyanate group.

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