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Modulating CO 2 Adsorption in Metal-Organic Frameworks via Metal-Ion Doping.
Inorganic Chemistry 2018 May 22
One novel metal-organic framework {[Ni6 (OH)4 (BTB)8/3 (H2 O)6 ]·4H2 O·9DMF} n (DMF = dimethylformamide) based on 1,3,5-benzenetribenzoic acid (H3 BTB) was successfully synthesized under basic condition at room temperature, featuring a unique twofold interpenetrated pcu-type net with [Ni6 (OH)4 (COO)8 (H2 O)6 ] cluster as building block. Its gas-adsorption behaviors were investigated and modified by utilizing metalII -doped procedure, which was certified to be a highly effective pathway in enhancing CO2 uptake capacity.
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