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Research Support, Non-U.S. Gov't
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α-Aminoalkyl Radical Addition to Maleimides via Electron Donor-Acceptor Complexes.

Chien-Wei Hsu, Henrik Sundén
Organic Letters 2018 April 7
A catalyst-free, photochemical oxidative annulation reaction between dialkylanilines and maleimides to generate tetrahydroquinolines is presented. The reaction is driven by the photochemical activity of an electron donor-acceptor (EDA) complex and has a broad substrate scope with the corresponding products isolated in good to excellent yields. Photochemical characterization of the EDA complex and a mechanistic rational is provided.

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