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Journal Article
Research Support, Non-U.S. Gov't
Dendrite-Free Li-Metal Battery Enabled by a Thin Asymmetric Solid Electrolyte with Engineered Layers.
Journal of the American Chemical Society 2018 January 11
The key bottleneck troubling the application of solid electrolyte is the contradictory requirements from Li-metal and cathode, which need high modulus to block Li-dendrite penetration and flexibility to enable low interface resistance, respectively. This study describes a thin asymmetrical design of solid electrolyte to address these shortcomings. In this architecture, a rigid ceramic-layer modified with an ultrathin polymer is toward Li-metal to accomplish dendrite-suppression of Li-anode, and a soft polymer-layer spreads over the exterior and interior of cathode to endow connected interface simultaneously. This ingenious arrangement endows solid Li-metal batteries with extremely high Coulombic efficiency and cyclability. This work will open up one avenue for realizing safe and long-life energy storage systems.
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