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Deliberately Designed Atomic-Level Silver-Containing Interface Results in Improved Rate Capability and Utilization of Silver Hollandite for Lithium-Ion Storage.
ACS Applied Materials & Interfaces 2018 January 11
α-MnO2 -structured materials are generally classified as semiconductors; thus, we present a strategy to increase electrochemical utilization through the design of a conductive material interface. Surface treatment of silver hollandite (Agx Mn8 O16 ) with Ag+ (Ag2 O) provides significant benefits to the resultant electrochemistry, including a decreased charge-transfer resistance and a 2-fold increase in deliverable energy density at a high rate. The improved function of this designed interface relative to conventional electrode fabrication strategies is highlighted.
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