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Journal Article
Research Support, Non-U.S. Gov't
Research Support, U.S. Gov't, Non-P.H.S.
Cooperative Electrocatalytic O 2 Reduction Involving Co(salophen) with p-Hydroquinone as an Electron-Proton Transfer Mediator.
Journal of the American Chemical Society 2017 December 28
The molecular cobalt complex, Co(salophen), and para-hydroquinone (H2 Q) serve as effective cocatalysts for the electrochemical reduction of O2 to water. Mechanistic studies reveal redox cooperativity between Co(salophen) and H2 Q. H2 Q serves as an electron-proton transfer mediator (EPTM) that enables electrochemical O2 reduction at higher potentials and with faster rates than is observed with Co(salophen) alone. Replacement of H2 Q with the higher-potential EPTM, 2-chloro-H2 Q, allows for faster O2 reduction rates at higher applied potential. These results demonstrate a unique strategy to achieve improved performance with molecular electrocatalyst systems.
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