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Angular-dependent magnetoresistance study in Ca<sub>0.73</sub>La<sub>0.27</sub>FeAs<sub>2</sub>: a "<i>parent</i>" compound of 112-type iron pnictide superconductors.

We report a study of angular-dependent magnetoresistance (AMR) with the magnetic field rotated in the plane perpendicular to the current on a Ca<sub>0.73</sub>La<sub>0.27</sub>FeAs<sub>2</sub> single crystal, which is regarded as a "<i>parent</i>" compound of 112-type iron pnictide superconductors. A pronounced AMR with twofold symmetry is observed, signifying the highly anisotropic Fermi surface. By further analyzing the AMR data, we find that the Fermi surface above the structural/antiferromagnetic (AFM) transition (<i>T</i><sub>s</sub>/<i>T</i><sub>N</sub>) is quasi-two-dimensional (2D), as revealed by the 2D scaling behavior of the AMR, Δρ/ρ(0) (<i>H</i>, θ)=Δρ/ρ(0) (μ<sub>0</sub><i>H</i>cos<i>θ</i>), <i>θ</i> being the magnetic field angle with respect to the c axis. While such a 2D scaling becomes invalid at temperatures below <i>T</i><sub>s</sub>/<i>T</i><sub>N</sub>, the three-dimensional (3D) scaling approach by inclusion of the anisotropy of Fermi surface is efficient, indicating that the appearance of 3D Fermi surface contributed to the anisotropic electronic transport. Compared with other experimental observations, we suspect that the additional 3D hole pocket (generated by the Ca <i>d</i> orbital and As1 <i>p</i><sub>z</sub> orbital) around the<i> Γ</i> point in CaFeAs<sub>2</sub> will disappear in the heavily electron doped regime, and moreover, the Fermi surface should be reconstructed across the structural/AFM transition. Besides, a quasi-linear in-plane magnetoresistance is observed at low temperatures and its possible origins are also discussed. Our results provide more information to further understand the electronic structure of 112-type IBSs.

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