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JOURNAL ARTICLE
RESEARCH SUPPORT, NON-U.S. GOV'T
Transition-Metal-Free Intermolecular α-Arylation of Ketones via Enolonium Species.
Organic Letters 2017 December 2
Herein it is shown, for the first time, that enolonium species are powerful electrophiles capable of reacting with aromatic compounds in an intermolecular manner to afford α-arylated ketones. The reaction is compatible with a variety of functional groups, is of wide scope with respect to aromatic compounds and ketone, and even works for polymerization-prone substrates such as substituted pyrroles, thiophenes, and furans. Only 1.6 to 5 equiv of the commodity aromatic substrates is needed.
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