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Heterostructured Arrays of Ni x P/S/Se Nanosheets on Co x P/S/Se Nanowires for Efficient Hydrogen Evolution.
ACS Applied Materials & Interfaces 2017 November 30
The development of efficient electrocatalysts for hydrogen evolution reaction (HER) is of increasing importance in energy conversion schemes. The earth-abundant transition-metal phosphides, especially CoP and Ni2 P, have emerged as promising catalysts for HER. We describe here the preparation and characterization of a hybrid catalyst of Ni2 P nanosheets@CoP nanowires on a carbon cloth for the reaction. The heterostructure and synergistic effects of the Ni2 P and CoP components result in an extremely low overpotential of 55 mV for achieving a catalytic current density of 10 mA cm-2 , which is remarkable for transition-metal phosphide electrocatalysts. The synthetic procedure could be readily extended to related, heterostructured bimetallic sulfides or selenides for HER.
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