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Methylene C(sp 3 )-H Arylation of Aliphatic Ketones Using a Transient Directing Group.
ACS Catalysis 2017 October 7
Palladium-catalyzed methylene β-C(sp3 )-H arylation of aliphatic ketones using a transient directing group is developed. The use of α-benzyl β-alanine directing group that forms a six-membered chelation with palladium is crucial for promoting the methylene C(sp3 )-H bond activation.
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