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Chloride-Tolerant Gold(I)-Catalyzed Regioselective Hydrochlorination of Alkynes.
ACS Catalysis 2017 October 7
We have developed a highly regioselective homogeneous gold(I)-catalyzed anti -hydrochlorination of unactivated alkynes at room temperature. We have overcome the incompatibility between conventional cationic gold catalysts and chloride by using a hydrogen-bonding activation of the Au-Cl bond. This approach is scalable, exhibits excellent functional group tolerance, and can be conducted in open air.
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