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Accessing Two-Coordinate Zn II Organocations by NHC Coordination: Synthesis, Structure, and Use as π-Lewis Acids in Alkene, Alkyne, and CO 2 Hydrosilylation.
Chemistry : a European Journal 2017 November 14
Discrete two-coordinate ZnII organocations of the type (NHC)Zn-R+ are reported, thanks to NHC stabilization. In preliminary reactivity studies, such entities, which are direct cationic analogues of long-known ZnR2 species, act as effective and tunable π-Lewis acid catalysts in alkene, alkyne, and CO2 hydrosilylation.
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