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Journal Article
Research Support, Non-U.S. Gov't
Synthesis and Characterization of Contorted Pentabenzo-Fused Coronenes as Semiconducting Materials.
Journal of Organic Chemistry 2017 August 5
Here, we report the synthesis and characterization of a series of contorted, yet noncentrosymmetrical, polycyclic aromatic hydrocarbons with a pentabenzo-fused coronene as the core framework. The parent pentabenzo[a,d,g,j,m]coronene (PBC) compound is shown to exhibit a shifted and rotated type of π-π stacking interactions, which render this series a semiconducting material. Single-crystal-based field-effect transistor devices of PBC exhibited efficient charge transport behavior, giving a p-channel field-effect mobility of 0.42 cm2 V-1 s-1 and an on/off ratio of 105 .
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