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Catalytic Enantioselective Reaction of Allenylnitriles with Imines Using Chiral Bis(imidazoline)s Palladium(II) Pincer Complexes.

Masaru Kondo, Masashi Omori, Tsubasa Hatanaka, Yasuhiro Funahashi, Shuichi Nakamura
Angewandte Chemie 2017 June 20
The first highly enantioselective reaction of allenylnitriles with imines has been developed. Excellent yields and enantioselectivities were observed for the reaction with various imines using chiral Phebim-Pd(II) complexes. This process offers a simple and efficient synthetic route for various functionalized α-vinylidene-β-aminonitriles and their derivatives.

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