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Transient process spectroscopy for the direct observation of inter-molecular photo-dissociation.
Structural Dynamics (Melville, N.Y.) 2017 September
Transient process spectroscopy has previously been thought to be applicable only to the analysis of intra-molecular processes. Two metal ion bridges used in the present work have allowed us to visualize real-time variations of the molecular vibration frequencies during photo-disproportionation inside bimolecule aggregates, which directly shows transient inter-molecular reactions.
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