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Aqueous Oxidations Started by TiO 2 Photoinduced Holes Can Be a Rate-Determining Step.
Chemistry, An Asian Journal 2017 August 18
In aqueous TiO2 photocatalytic hydroxylation of weakly polar aromatics, a series of inverse H/D KIEs of 0.7-0.8 were observed, which is different than the normal H/D kinetic isotope effects (KIEs) usually observed for polar aromatics. This result indicated that the oxidation started by photo-induced hvb + can be the rate-determining step.
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