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Reversible conversion between a pleated oligo-tetrathiafulvalene radical foldamer and folded donor-acceptor [3]pseudorotaxane under redox conditions.
Chemical Communications : Chem Comm 2017 May 12
Linear tetrathiafulvalene (TTF) oligomers were synthesized, which could not only form a pleated TTF˙+ radical cation foldamer under oxidation conditions, but also interlocked with CBPQT4+ to form folded donor-acceptor [3]pseudorotaxane in the neutral state of TTF. Moreover, switchable transformation between these two folded supramolecular structures was achieved under the alternative regulation of the redox states of TTF units.
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