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High and Selective Carbon Dioxide Capture in Nitrogen-Containing Aerogels via Synergistic Effects of Electrostatic In-Plane and Dispersive π-π-Stacking Interactions.
ACS Applied Materials & Interfaces 2017 May 11
A new strategy for CO2 capture is reported based on the synergistic effect of electrostatic in-plane and dispersive π-π-stacking interactions of amide and indole with CO2 . Density functional theory illustrated that the amide group can have an increased ability to capture CO2 molecules that were just desorbed from an adjacent indole unit. We used this strategy to fabricate a microporous aerogel that exhibited a superior CO2 capture performance in both dry and wet conditions. The proposed synergistic effect is expected to be a new rationale for the design of CO2 capture materials.
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