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Binding CO2 by a Cr8 Metallacrown.
Angewandte Chemie 2017 May 9
The {Cr8 } metallacrown [CrF(O2 C(t) Bu)2 ]8 , containing a F-lined internal cavity, shows high selectivity for CO2 over N2 . DFT calculations and absorption studies support the multiple binding of F-groups to the C-center of CO2 (C⋅⋅⋅F 3.190(9)-3.389(9) Å), as confirmed by single-crystal X-ray diffraction.
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