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Synthesis of Aromatic Sulfones from SO2 and Organosilanes Under Metal-free Conditions.

Niklas von Wolff, Joëlle Char, Xavier Frogneux, Thibault Cantat
Angewandte Chemie 2017 May 9
The conversion of SO2 into arylsulfones under metal-free conditions was achieved for the first time by reacting SO2 with (hetero)arylsilanes and alkylhalides in the presence of a fluoride source. The mechanism of this transformation was elucidated based on DFT calculations, which highlight the influence of SO2 in promoting C-Si bond cleavage.

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