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Synthesis, Structures, and Photophysical Properties of Alternating Donor-Acceptor Cycloparaphenylenes.
Chemistry : a European Journal 2017 May 30
The synthesis of alternating donor-acceptor [12] and [16]cycloparaphenylenes (CPPs) has been achieved by the rhodium-catalyzed intermolecular cross-cyclotrimerization followed by imidation and/or aromatization. These alternating donor-acceptor CPPs showed positive solvatofluorochromic properties and smaller HOMO-LUMO gaps compared with nonfunctionalized CPPs, which was confirmed by the theoretical study.
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