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JOURNAL ARTICLE
RESEARCH SUPPORT, NON-U.S. GOV'T
Gas-Phase Photochemical Overall H 2 S Splitting by UV Light Irradiation.
ChemSusChem 2017 May 10
Splitting of hydrogen sulfide is achieved to produce value-added chemicals. Upon irradiation at 254 nm in the gas phase and in the absence of catalysts or photocatalysts at near room temperature, H2 S splits into stoichiometric amounts of H2 and S with a quantum efficiency close to 50 %. No influence of the presence of CH4 and CO2 (typical components in natural gas and biogas in which H2 S is an unwanted component) on the efficiency of overall H2 S splitting was observed. A mechanism for the H2 and S formation is proposed.
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