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Lasing behavior of surface functionalized carbon quantum dot/RhB composites.
Nanoscale 2017 April 21
Random lasers have been extensively and intensively investigated due to their fundamental importance and promising applications. Here, we explored the lasing behavior of carbon quantum dot (CQD)/Rhodamine B (RhB) composites. CQDs exhibited a broad emission spectrum which overlapped with the absorption spectrum of the RhB dye. We investigated an approach wherein the -OH, -NH2 and -PO4 group functionalized CQD/RhB composites showed lasing behavior. The optical pumping of functionalized CQD/RhB composites exhibited lasing emission which is dynamically tunable as a function of the surface properties of CQDs at the laser wavelength of 532 nm by varying the pump energy. The PO4 -CQD/RhB composites showed a typical lasing emission with a linewidth of 3.2 nm at 587 nm at 1.86 mJ pump energy. We also demonstrated that the pH value of CQD solution played a key role on the lasing behavior of CQD/composites.
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