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Electrocatalytic water oxidation by copper(ii) complexes containing a tetra- or pentadentate amine-pyridine ligand.
Chemical Communications : Chem Comm 2017 April 22
Two water soluble copper(ii) complexes containing amine-pyridine ligands were found to be catalytically active for water oxidation reactions in basic solutions, with observed rate constants of 13.1-18.7 s-1 . These complexes are robust in basic solutions and displayed good stability over 5 h of electrolysis in pH 11.5 phosphate buffer at 1.4 V vs. NHE.
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