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The Nickel-Pincer Complex in Lactate Racemase Is an Electron Relay and Sink that acts through Proton-Coupled Electron Transfer.
Angewandte Chemie 2017 Februrary 4
QM/MM calculations reveal that the nickel pincer complex in lactate racemase functions as a reversible "single-center electrode" that accepts and donates back an electron. In this way, it catalyzes the isomerization process d-lactate⇌l-lactate through successive proton-coupled electron-transfer steps.
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