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Journal Article
Research Support, U.S. Gov't, Non-P.H.S.
Atomic Number Dependent "Structural Transitions" in Ordered Lanthanide Monolayers: Role of the Hydration Shell.
Langmuir : the ACS Journal of Surfaces and Colloids 2017 Februrary 15
When lanthanide ions are present in the aqueous subphase of a floating monolayer (Langmuir film), the ions attracted to the interface will in many cases form commensurate and/or incommensurate two-dimensional structures. These lattices depend not only on the molecules forming the monolayer, but also on the atomic number of the lanthanide, with a sudden change between the lattice formed by lighter ions and that formed by heavier ions under a given monolayer. Since there are few other relevant differences between the lanthanides, we attribute the Z-dependent "transition" to the number of water molecules associated with each ion. The first hydration shell is thought to vary continuously from ∼9 in lighter lanthanides to ∼8 in heavier lanthanides.
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