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Chemically reversible binding of H 2 S to a zinc porphyrin complex: towards implementation of a reversible sensor via a "coordinative-based approach".
Dalton Transactions : An International Journal of Inorganic Chemistry 2017 Februrary 15
Binding of hydrogen sulfide (H2 S) to a zinc porphyrin complex and the stabilization of the related zinc hydrosulfido adduct are explored. High-resolution MALDI Fourier transform ion cyclotron resonance mass spectrometry (HR MALDI-FT-ICR) and1 H NMR experiments provide evidence that HS- coordination occurs at the zinc centre. The coordination of HS- occurs in a reversible manner and modulates fluorescence emission of a tetra(N-methylpyridyl)porphine zinc complex (TMPyPZn). The results highlight the potential of TMPyPZn and related systems for the implementation of fast and simple H2 S sensors via a coordinative-based approach.
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