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Spin-Lattice Coupling in [Ni(HF 2 )(pyrazine) 2 ]SbF 6 Involving the HF 2 - Superexchange Pathway.
Inorganic Chemistry 2016 December 6
Magnetoelastic coupling in the quantum magnet [Ni(HF2 )(pyrazine)2 ]SbF6 has been investigated via vibrational spectroscopy using temperature, magnetic field, and pressure as tuning parameters. While pyrazine is known to be a malleable magnetic superexchange ligand, we find that HF2 - is surprisingly sensitive to external stimuli and is actively involved in both the magnetic quantum phase transition and the series of pressure-induced structural distortions. The amplified spin-lattice interactions involving the bifluoride ligand can be understood in terms of the relative importance of the intra- and interplanar magnetic energy scales.
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