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JOURNAL ARTICLE
RESEARCH SUPPORT, NON-U.S. GOV'T
High-Performance Porphyrin-Based Dye-Sensitized Solar Cells with Iodine and Cobalt Redox Shuttles.
ChemSusChem 2017 March 10
Recently, enormous research passion has been devoted to enhance the power conversion efficiency (PCE) of porphyrin sensitizers for dye-sensitized solar cells (DSSCs), but the major stumbling block is the absorption defect in the visible-light region. To address this challenge, high-performance DSSCs are reported based on a new donor-π-acceptor sensitizer FW-1, 7H-dibenzo[c,g]carbazole-substituted and fused zinc porphyrin, co-sensitized with a benzotriazole-containing dye (WS-5) in iodine and cobalt redox systems, and high PCEs of 10.21 and 10.42 %, respectively, were obtained. An unprecedented breakthrough was obtained by making one sensitizer suitable for several electrolyte systems because of its appropriate molecular orbitals and co-sensitizer.
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