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Asymmetric Synthesis by Using Natural Sunlight under Absolute Achiral Conditions.
Chemistry : a European Journal 2017 January 32
Irradiation of prochiral (E)-aroylacrylamide with sunlight gave single-handed pyrrolinone quantitatively and with an enantiomeric excess (ee) of over 99 % under absolutely achiral conditions. The phenomenon was explained by photoisomerization and reversible cyclization followed by dynamic crystallization involving deracemization.
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