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Alkyl Side-Chain Engineering in Wide-Bandgap Copolymers Leading to Power Conversion Efficiencies over 10.

Tao Liu, Xuexue Pan, Xiangyi Meng, Yu Liu, Donghui Wei, Wei Ma, Lijun Huo, Xiaobo Sun, Tack Ho Lee, Minjuan Huang, Hyosung Choi, Jin Young Kim, Wallace C H Choy, Yanming Sun
Advanced Materials 2017 Februrary
A series of wide-bandgap (WBG) copolymers with different alkyl side chains are synthesized. Among them, copolymer PBT1-EH with moderatly bulky side chains on the acceptor unit shows the best photovoltaic performance with power conversion efficiency over 10%. The results suggest that the alkyl side-chain engineering is an effective strategy to further tuning the optoelectronic properties of WBG copolymers.

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