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Branched 1,2,3-Triazolium-Functionalized Polyacetylene with Enhanced Conductivity.
Macromolecular Rapid Communications 2016 December
Metathesis cyclopolymerization of mono- or bissubstituted 1,6-heptadiynes is undergone to generate the ionic polyacetylenes (iPAs) with branched 1,2,3-ttriazolium pendants, which possess relatively high intrinsic ionic conductivities of 1.4 × 10(-5) -2.1 × 10(-5) S cm(-1) at 30 °C. The doping treatment with lithium bis(trifluoromethanesulfonyl)imide endows iPAs with enhanced ionic conductivities of 2.5 × 10(-5) -4.3 × 10(-5) S cm(-1) . Further doping with iodine, iPAs show ionic and electronic dual conductivities of 4.5 × 10(-5) -7.1 × 10(-4) and 1.5 × 10(-6) -4.5 × 10(-6) S cm(-1) , respectively. Therefore, the doped iPAs demonstrate the potential in the area of conducting polymers and polymeric electronics.
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