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Designing isometrical gel precursors to identify the gelation pathway for nickel-selective metallohydrogels.
Two novel multi-responsive metallohydrogels, namely, 2-PF-Ni and 3-PF-Ni, were successfully constructed from phenylalanine derivatives. The 2-PF gelator shows specific responses to Ni2+ ; particularly, 2-PF-Ni is lavender colored, which has been rarely reported among hydrogels triggered by Ni2+ . 3-PF-Ni is light green and exhibits perfect thixotropy. This paper provides insights into the gelation mechanisms of these two metallogels.
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