Atomically Dispersed Ru on Ultrathin Pd Nanoribbons.

JingJie Ge, Dong Sheng He, Wenxing Chen, Huanxin Ju, Han Zhang, Tingting Chao, Xiaoqian Wang, Rui You, Yue Lin, Yu Wang, Junfa Zhu, Hai Li, Bin Xiao, Weixin Huang, Yuen Wu, Xun Hong, Yadong Li

Journal of the American Chemical Society 2016 October 15

We report a one-pot synthesis of atomically dispersed Ru on ultrathin Pd nanoribbons. By using synchrotron radiation photoemission spectroscopy (SRPES), extended X-ray absorption fine structure (EXAFS) measurements in combination with aberration corrected high-resolution transmission electron microscopy (HRTEM), we show that atomically dispersed Ru with content up to 5.9% was on the surface of the ultrathin nanoribbon. Furthermore, the ultrathin Pd/Ru nanoribbons could remarkably prohibited the hydrogenolysis in chemoselective hydrogenation of C=C bonds, leading to an excellent catalytic selectivity compared with the commercial Pd/C and Ru/C.

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