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A binary catalyst system of a cationic Ru-CNC pincer complex with an alkali metal salt for selective hydroboration of carbon dioxide.

Chee Koon Ng, Jie Wu, T S Andy Hor, He-Kuan Luo
Chemical Communications : Chem Comm 2016 September 28
Binary catalyst systems comprising a cationic Ru-CNC pincer complex and an alkali metal salt were developed for selective hydroboration of CO2 utilizing pinacolborane at r.t. and 1 atm CO2 , with the combination of [Ru(CNCBn )(CO)2 (H)][PF6 ] and KOCO2 t Bu producing formoxyborane in 76% yield. A bicyclic catalytic mechanism was proposed and discussed.

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