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Diverse reactivity of borenium cations with >N-H compounds.
Chemical Communications : Chem Comm 2016 July 8
The Ph2P-stabilized borenium reacts cleanly with PhNH2, NH3 and HNTf2 to give a variety of boron compounds, namely the amino-substituted borenium (substitution reaction at B), the neutral phosphine-borane , the mixed P/N-stabilized boronium and the dicationic boron species . Remote modulation of the Lewis acidity at boron has been studied by preparing the related iPr2P-stabilized borenium and reacting it with dihydrogen.
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