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Magnetic frustration in a hexaazatrinaphthylene-bridged trimetallic dysprosium single-molecule magnet.
The synthesis, structure and magnetic properties of the HAN-bridged tri-dysprosium complex [{(thd)3 Dy}3 HAN] (1) are described. The complex is an SMM that shows two relaxation processes owing to the presence of two geometrically distinct Dy3+ sites in 1. Ab initio calculations reveal that the magnetic ground state of 1 is characterized by magnetic frustration.
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