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A simple approach to hybrid inorganic-organic step-growth hydrogels with scalable control of physicochemical properties and biodegradability.
Polymer Chemistry 2015 March 29
We prepared new and scalable, hybrid inorganic-organic step-growth hydrogels with polyhedral oligomeric silsesquioxane (POSS) network knot construction elements and hydrolytically degradable poly(ethylene glycol) (PEG) di-ester macromonomers by in situ radical-mediated thiol-ene photopolymerization. The physicochemical properties of the gels are fine-tailored over orders of magnitude including functionalization of their interior, a hierarchical gel structure, and biodegradability.
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